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Deterioration in fuel cell performance resulting from hydrogen fuel containing impurities: poisoning effects by CO,CH4, HCHO and HCOOH
Institution:1. Environment and Energy Research Division, National Traffic Safety and Environment Laboratory (NTSEL), 7-42-27,Jindaiji-higashi-machi, Chofu, Tokyo 182-0012, Japan;2. Technical Education Department, Environment & Energy Laboratory, Gunma University, 4-2 Aramaki, Maebashi, Gunma 371-8510, Japan;3. Department of Mechanical Engineering, Faculty of Engineering, Kokushikan University, 4-28-1, Setagaya, Setagaya-ku, Tokyo 154-8515, Japan;1. German Aerospace Center, Institute of Engineering Thermodynamics, Germany;2. German Aerospace Center, Institute of Networked Energy Systems, Germany;1. Department of Chemistry, Imperial College London, London SW7 2AZ, UK;2. Centre for Fuel Cell Technology, ARCI, Taramani, Chennai 600 113, India;1. Department of Chemistry, Imperial College London, London SW7 2AZ, UK;2. Department of Energy, Tezpur University, Tezpur 784 028, India;1. Hawaii Natural Energy Institute, University of Hawaii, Honolulu, HI, 96822, USA;2. Center for Microengineered Materials, University of New Mexico, Albuquerque, NM, 87131, USA
Abstract:This paper covers our investigation into a decline in fuel cell (FC) performance resulting from hydrogen fuel containing impurities. This is a serious problem in case of adopting the methanol or gasoline reforming approach as a means of supplying fuel to FCs. The results are summarized as follows:(1) Components of the gas generated by the reformer adopting the steam reforming and auto thermal reforming approach were predicted and specific components and concentrations were identified;(2) Various experiments and analyses were conducted to determine the adverse effect of CO, CH4, HCHO and HCOOH poisoning on the performance of FC.
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