PM2.5 and NOx from traffic: Human health impacts,external costs and policy implications from the Belgian perspective

This article employs an optimized impact pathway approach to marginal external health costs that relies on high-resolution dispersion models calibrated for Belgium and the surrounding areas. Per tonne, the MEHC_PM2.5 is found to be many times larger than MEHC_NOx, which is currently negative. Further, the impact of Belgian PM_2.5 emissions in the immediate area of generation is significantly larger than the impact on more distant areas; the opposite is true for NO_x. The MEHCs of both pollutants are predicted to increase in the coming years. Further analysis of the impacts of PM_2.5 and NO_x reveals that, on average, modern gasoline vehicles outperform their diesel counterparts as far as future emissions are concerned. This contrasts with findings for 2007, which suggested that Euro 5 diesels had fewer associated health costs because of the potential for ozone reduction offered by their NO_x emissions.     

Costs of air pollutants from shipping: a meta-regression analysis

ABSTRACT

This study estimated the external cost of air pollution from shipping by means of a meta-regression analysis, which has not been made before. Three pollutants, which were included in most of the primary studies, were considered: nitrogen oxides (NO_x), sulphur dioxides (SO₂) and particulate matters with a diameter of max 2.5 micrometres (PM_2.5). All primary studies included damages of health and a majority added impacts on agriculture and estimated the cost of air pollutants by transferring cost estimates from studies on costs of air emissions from transports in Europe. Different regression models and estimators were used and robust results were found of statistically significant emission elasticities of below one, i.e. total external costs increase by less than 1% when emissions increase by 1%. There was a small variation between the pollutants, with the highest elasticity for PM_2.5 and lowest for NO_x. Calculations of the marginal external cost of the pollutants showed the same pattern, with this cost being approximately six times higher for PM_2.5 than for the other pollutants. Common to all pollutants was that the marginal external cost decreases when emission increases. Another robust result was a significant increase in the cost of studies published in journals compared with other publication outlets. These findings point out some caution when transferring constant external unit cost of air pollutant from shipping, which is much applied in the literature, and the cost functions estimated in this study could thus provide a complementary transfer mechanism.     

Cruise activity and pollution: The case of Barcelona

One of the main causes of mortality worldwide is air pollution. To tackle this problem, local, regional and national governments have implemented policies to reduce emissions from industrial and on-road sources. However, when these policies are being designed, shipping emissions are often overlooked. There has been a drastic increase in the demand for cruises and its economic relevance is also growing in port-cities. Barcelona is Europe’s leading cruise port, and it is located near the centre of the city. In this context, this paper analyses the impact of cruise ships in the air quality of the entire city of Barcelona using a dataset with information about pollutants and the number of cruises arriving to the port. We show that there is a direct impact between cruises staying at the port and city pollution. Additionally, the size and age of the cruise also affect air quality. The larger (or newer) the cruise is, the higher the emission generated. Moreover, our simulations show that the whole city is affected by these emissions.     

Identifying contributions of on-road motor vehicles to urban air pollution using travel demand model data

Ambient concentrations of pollutants are correlated with emissions, but the contribution to ambient air quality of on-road mobile sources is not necessarily equal to their contribution to regional emissions. This is true for several reasons such as the distribution of other pollution sources and regional topology, as well as meteorology. In this paper, using a dataset from a travel demand model for the Sacramento metropolitan area for 2005, regional vehicle emissions are disaggregated into hourly, gridded emission inventories, and transportation-related concentrations are estimated using an atmospheric dispersion model. Contributions of on-road motor vehicles to urban air pollution are then identified at a regional scale. The contributions to ambient concentrations are slightly higher than emission fractions that transportation accounts for in the region, reflecting that relative to other major pollution sources, mobile sources tend to have a close proximity to air quality monitors in urban areas. The contribution results indicate that the impact of mobile sources on PM₁₀ is not negligible, and mobile sources have a significant influence on both NO_x and VOC pollution that subsequently results in secondary particulate matter and ozone formation.     

Atmospheric Emissions from Shipping: The Need for Regulation and Approaches to Compliance

Shipping has traditionally been viewed as the least environmentally damaging mode of freight transport. Recent studies have increasingly questioned this perception, as attention has focused on both the greenhouse gas emissions (mainly CO₂) and the emission of health-damaging pollutants (such as sulphur, nitrogen oxides and particulates) by ships. This paper reviews the available evidence on the atmospheric emissions of shipping. It proposes that the profit objective has prompted the pursuit of greater fuel efficiency within the sector, but that reliance on market forces alone is insufficient to deliver on the environmental imperative. The paper outlines the current and planned regulatory regime for the atmospheric emissions from ships and posits that greater, and more diverse, market regulation is required. Alternative general approaches to regulatory compliance are categorised as ‘alternative sources of energy’ or ‘abatement technologies’ and the characteristics of a range of specific options are analysed. The paper concludes that although the shipping industry has been slow to improve its environmental credentials, a combination of regulation and technological innovation provides it with significant potential to dramatically reduce its environmental impact.     

Port-city exhaust emission model: An application to cruise and ferry operations in Las Palmas Port

Exhaust emissions cause air pollution and climate change. The exhausts of shipboard fuel combustion are equally damaging particularly, so close to the environmentally sensitive mainland and island coasts, as well as at ports due to their urbanized character. This paper estimates, for the first time, exhaust pollutants related to cruise and ferry operations in Las Palmas Port and, in an island context. Emission assessment is based on a full bottom-up model and messages transmitted by the Automatic Identification System during 2011. Results are described as a breakdown of NOx, SOx, PM_2.5, CO and CO₂, according to ship classes, operative type and time, providing valuable information to environmental policy makers in port-city areas and islands under similar conditions. It is generally concluded that vessel traffic and passenger shipping in particular are a source of air pollution in Las Palmas Port. Emission maps confirm location of hot spots in quays assigned for cruise and ferry operations. Policy recommendations encourage regular monitoring of exhaust emissions and market-based incentives supported by details on polluting and operative profiles. On the other hand, feasibility studies are suggested for automated mooring, LNG bunkering facilities and also shore-side energy services, prioritizing berthing of shipping sectors (or sub-sectors) with the highest share of exhaust emissions once their local effects have been confirmed by a dispersion, exposure and impact assessment.     

Personal exposures to PM during short distance highway travel in India

Traffic is the largest contributor (37%) to urban air pollution in India. During commuting, passengers are significantly exposed to pollutants. We carried out a study on a National Highway (NH) in India to measure personal exposure to Particulate Matter (PM) in five travel modes. PM_2.5 concentrations showed the following trend: Bus > Car FA (fresh air mode of air condition) > Bus AC > Car > Car RC (re-circulation mode of air condition). Highest and lowest concentrations of PM₁₀ were observed in Bus (134 ± 47 µg m⁻³) and Car RC (20 ± 5 µg m⁻³), respectively. The exposures were highest at the rear seats during the Bus AC journeys. In Car FA, the contribution of PM₁ to total concentrations was dominant (61%). Travel modes explained highest variabilities in PM₁₀, PM_2.5 and PM₁ concentrations. In all travel modes, the highest particle counts were observed for PM_0.3–0.5. PM_>0.5–5.0 counts during Bus journeys were comparatively higher than remaining modes. Deposition doses of passengers were as high as 3.22 µg of PM₁₀ (in Bus), 0.66 µg of PM_2.5 (in Bus) and 0.06 µg of PM₁ (in Bus AC) during the ~1 h journey. Our study revealed that Car RC is the safest mode of travel, both in terms of personal exposures and PM depositions in respiratory system. The results from this study can be used to target efforts to reduce personal exposure of highway commuters.     

Contrasting the direct use of data from traffic radars and video-cameras with traffic simulation in the estimation of road emissions and PM hotspot analysis

This study investigates the effect of traffic volume and speed data on the simulation of vehicle emissions and hotspot analysis. Data from a microwave radar and video cameras were first used directly for emission modelling. They were then used as input to a traffic simulation model whereby vehicle drive cycles were extracted to estimate emissions. To reach this objective, hourly traffic data were collected from three periods including morning peak (6–9 am), midday (11–2 pm), and afternoon peak (3–6 pm) on a weekday (June 23, 2016) along a high-volume corridor in Toronto, Canada. Traffic volumes were detected by a single radar and two video cameras operated by the Southern Ontario Centre for Atmospheric Aerosol Research. Traffic volume and composition derived from the radar had lower accuracy than the video camera data and the radar performance varied by lane exhibiting poorer performance in the remote lanes. Radar speeds collected at a single point on the corridor had higher variability than simulated traffic speeds, and average speeds were closer after model calibration. Traffic emissions of nitrogen oxides (NOx) and particulate matter (PM₁₀ and PM_2.5) were estimated using radar data as well as using simulated traffic based on various speed aggregation methods. Our results illustrate the range of emission estimates (NO_x: 4.0–27.0 g; PM₁₀: 0.3–4.8 g; PM_2.5: 0.2–1.3 g) for the corridor. The estimates based on radar speeds were at least three times lower than emissions derived from simulated vehicle trajectories. Finally, the PM₁₀ and PM_2.5 near-road concentrations derived from emissions based on simulated speeds were two or three times higher than concentrations based on emissions derived using radar data. Our findings are relevant for project-level emission inventories and PM hot-spot analysis; caution must be exercised when using raw radar data for emission modeling purposes.     

Particulate matter concentrations and heavy metal contamination levels in the railway transport system of Sydney,Australia

Sampling campaign was conducted over six weeks to determine particulate matter (PM) concentrations from Sydney Trains airport line (T2) at both underground and ground levels using DustTrak. Dust samples were collected and analysed for 12 metals (Fe, Ca, Mn, Cr, Zn, Cu, Pb, Al, Co, Ni, Ba and Na) by atomic emission spectroscopy. Average underground PM₁₀ and PM_2.5 concentrations from inside the trains were 2.8 and 2.5 times greater than at ground level. Similarly, PM₁₀ and PM_2.5 concentrations on underground platforms were 2.7 and 2.5 times greater than ground level platforms. Average underground PM concentrations exceeded the national air quality standards for both PM₁₀ (50 µg/m³) and PM_2.5 (25 µg/m³). Correlation analysis showed a strong to moderate association between PM concentrations at ground level and background PM concentrations (r² from 0.952 to 0.500). The findings suggested that underground PM concentrations were less influenced by the ambient background than at ground level. The metal concentrations decreased in the order of Fe, Cr, Ca, Al, Na, Ba, Mn, Zn, Cu, Ni, Co and Pb. The pollution index (PI) and enrichment factor (EF) values were calculated to identify the levels and sources of contamination in the underground railway microenvironments. PM was remarkably rich in Fe with a mean concentration of 73.51 mg/g and EF of 61.31, followed by Ni and Cr. These results noticeably indicated a high level of metal contamination in the underground environments, with the principal contribution from track abrasion and wear processes.     

Characteristics of particulate matter (PM) concentrations influenced by piston wind and train door opening in the Shanghai subway system

More than 9 million passengers take Shanghai’s subway system every work day. The system’s air quality has caused widespread concern because of the potential harm to passengers’ health. We measured the particulate matter (PM) concentrations at three kinds of typical underground platform (side-type, island-type, and stacked-type platforms) and inside the trains in Shanghai’s metro during 7 days of measurements in April and July 2015. Our results demonstrated that the patterns of air quality variation and PM concentrations were similar at the side-type and island-type platforms. We also found that the PM concentrations were higher on the platforms than inside the train and that the PM concentrations in the subway system were positively correlated with those in the ambient air. Piston wind generated by vehicle motion pushes air from the tunnel to the platform, so platform PM concentrations increase when trains approach the platform. However, the piston wind effect varies greatly between locations on the platform. In general, the effect of the piston wind is weaker at the middle of the platform than at both ends. PM concentrations inside the train increase after the doors open, during which time dirty platform air floods into the compartments. PM_1.0 and PM_2.5 were significantly correlated both inside the train and on the platforms. PM_1.0 accounted for 71.9% of PM_2.5 inside the train, which is higher than the corresponding platform values. Based on these results, we propose some practical suggestions to minimize air pollution damage to passengers and staff from the subway system.     

Impacts of fuel quality on indoor environment onboard a ship: From policy to practice

Environmental considerations, concerning the negative impacts of ship exhaust gases and particles on ambient air quality, are behind the requirements of cleaner marine fuels currently applied in designated emission control areas (ECAs). We investigated the impact of a ship operating on two types of fuel on the indoor air quality onboard. Gaseous and particulate air pollutants were measured in the engine room and the accommodation sections on-board an icebreaker operating first on Heavy Fuel Oil (HFO, 1%-S), and later Marine Diesel Oil (MDO, 0.1%-S). Statistically significant decrease of SO₂, NOx, PM_2.5 and particle number concentration were observed when the ship was operating on MDO. Due to the higher content of alkylated PAHs in MDO compared to HFO, the concentration of PAHs increased during operation on MDO. The particulate PAHs classified as carcinogens, were similar to or lower in the MDO campaign. Chemical analysis of PM_2.5 revealed that the particles consisted mainly of organic carbon and sulfate, although the fraction of metals was quite large in particles from the engine room. Principal Component Analysis of all measured parameters showed a clear difference between HFO and MDO fuel on the indoor environmental quality on-board the ship. This empirical study poses a first example on how environmental policy-making impacts not only the primary target at a global level, but also brings unexpected localized benefits at workplace level. The study emphasizes the need of further investigations on the impact of new marine fuels and technologies on the indoor air environments on board.     

Sources and exposure risk of trace elements for traffic policemen in roadside locations

Samples of PM_2.5 and PM₁₀ at four types of roadside location (major road, secondary road, branch road, and expressway) in Tianjin were collected and analyzed in 2015. The average annual roadside PM_2.5 and PM₁₀ concentrations were higher than the national ambient air quality standard (NAAQS: GB3095-2012). The chromium (Cr), manganese (Mn), nickel (Ni), zinc (Zn), arsenic (As), and cadmium (Cd) concentrations in both PM_2.5 and PM₁₀ over four seasons displayed significant differences (p < 0.05). An enrichment factor (EF) analysis revealed that Cd, copper (Cu), Zn, As, Ni, and Pb in PM_2.5 and PM₁₀ mainly originated from anthropogenic sources. A factor analysis (FA) and correlation analysis (CA) revealed that vehicle emissions (exhaust and non-exhaust), soil dust, coal combustion, and industrial emissions were the main sources of roadside PM_2.5 and PM₁₀ in Tianjin. Both the total hazard quotients (total HQ) and the total carcinogenic risk (total CR) for selected elements in PM_2.5 and PM₁₀ were within acceptable limits. The HQ of Pb was higher than for other metals, and it should therefore be given special attention. The CR for traffic policemen was highest for Cr exposure (1.01 × 10⁻⁵ for PM_2.5 and 1.52 × 10⁻⁵ for PM₁₀), followed by As and Ni. A sensitivity analysis showed that the total contributions of the metal concentrations, exposure time (ET), and exposure frequency (EF) accounted for over 50% of the risk for Cr, As, and Ni, suggesting that these metals had the greatest impact on the uncertainty of health risk assessments.     

Evaluating the social cost of cruise ships air emissions in major ports of Greece

Detailed NO_x, SO₂ and PM_2.5 emissions have been estimated for cruise ships in the five busiest Greek ports (i.e. Piraeus, Santorini, Mykonos, Corfu and Katakolo) for year 2013. The emissions were analyzed in terms of gas species, seasonality and activity. The total in-port inventory of cruise shipping accounted to 2742.7 tons: with NO_x being dominant (1887.5 tons), followed by SO₂ and PM_2.5 (760.9 and 94.3 tons respectively). Emissions during hotelling corresponded to 88.5% of total and have significantly outweighed those produced during ships’ maneuvering activities (11.5% of total). Seasonality was found to play a major role, as summer emissions and associated impacts were significantly augmented. The anticipated health impacts of ship emissions can reach to €24.3 million or to €5.3 per passenger proving the necessity of control of the emissions produced by cruise ships in port cities or policy and measures towards a more efficient cruise industry.     

Health externalities of ship air pollution at port – Piraeus port case study

This paper is employing the well-known methodology of impact pathway approach to assess the external costs in human health from ship air pollution at port areas. The passenger port of Piraeus, Greece is the scenery of the study. Piraeus port is in the vicinity of the greater Athens metropolitan area where almost half of the country’s population lives. Hence, this port is the central hub of the Greek coastal passenger ship system which connects the islands of the Aegean Sea with land and is characterized by heavy ship traffic. The case study presented in this paper assesses the annual external cost in human health from air emissions produced by all passenger ships and cruise ships calling the port of Piraeus. Health cost from ships at port has been estimated at both local (Athens metropolitan area) and regional level (entire territory of Greece). Results show that higher costs occur at the local level. The dominant pollutants creating this cost are particulate matter (PM_2.5, and PM₁₀). Overall, the results indicate that the health impact of Piraeus’s passenger port emissions is not negligible; however the cost of PM₁₀ is considerably lower than the corresponded cost deriving from the land based industries of the Athens regional area for which comparison has been available.     

Long-term behavior of particulate matters at urban roadside and background locations in Seoul,Korea

The concentrations of particulate matter, PM_2.5, PM₁₀, and TSP at an urban roadside and an urban background station are analyzed. Data collected over a 10 year period are analyzed. The concentrations of the particulates measured at the urban site are systematically larger than at the background station. The mean PM values at the former also exhibit a slight fall over the decade unlike those at the background station. Overall, the particulate matters at both locations are in an intermediate range of global level, e.g., approximately two times lower than those in other Asian regions but higher than in Europe.     

Integrated data-driven modeling to estimate PM2.5 pollution from heavy-duty truck transportation activity over metropolitan area

Based on the national emission inventory data from different countries, heavy-duty trucks are the highest on-road PM_2.5 emitters and their representation is estimated disproportionately using current modeling methods. This study expands current understanding of the impact of heavy-duty truck movement on the overall PM_2.5 pollution in urban areas through an integrated data-driven modeling methodology that could more closely represent the truck transportation activities. A detailed integrated modeling methodology is presented in the paper to estimate urban truck related PM_2.5 pollution by using a robust spatial regression-based truck activity model, the mobile source emission and Gaussian dispersion models. In this research, finely resolved spatial–temporal emissions were calculated using bottom-up approach, where hourly truck activity and detailed truck-class specific emissions rates are used as inputs. To validate the proposed methodology, the Cincinnati urban area was selected as a case study site and the proposed truck model was used with U.S. EPA’s MOVES and AERMOD models. The heavy-duty truck released PM_2.5 pollution is estimated using observed concentrations at the urban air quality monitoring stations. The monthly air quality trend estimated using our methodology matches very well with the observed trend at two different continuous monitoring stations with Spearman’s rank correlation coefficient of 0.885. Based on emission model results, it is found that 71 percent of the urban mobile-source PM_2.5 emissions are caused by trucks and also 21 percent of the urban overall ambient PM_2.5 concentrations can be attributed to trucks in Cincinnati urban area.     

Congestion and emissions mitigation: A comparison of capacity,demand, and vehicle based strategies

Capacity, demand, and vehicle based emissions reduction strategies are compared for several pollutants employing aggregate US congestion and vehicle fleet condition data. We find that congestion mitigation does not inevitably lead to reduced emissions; the net effect of mitigation depends on the balance of induced travel demand and increased vehicle efficiency that in turn depend on the pollutant, congestion level, and fleet composition. In the long run, capacity-based congestion improvements within certain speed intervals can reasonably be expected to increase emissions of CO₂e, CO, and NO_x through increased vehicle travel volume. Better opportunities for emissions reductions exist for HC and PM_2.5 emissions, and on more heavily congested arterials. Advanced-efficiency vehicles with emissions rates that are less sensitive to congestion than conventional vehicles generate less emissions co-benefits from congestion mitigation.     

Natural variability in exposure to fine particles and their trace elements during typical workdays in an urban area

Studies on the natural human exposures to fine particulate matter (PM_2.5) and their elements composition are practically non-existent in South America. In order to understand the natural exposure of the typical Brazilian population to PM_2.5 and their trace element composition, we measured PM_2.5 concentrations and collected mass on filters for nine continuous hours during a typical workday of volunteers. In addition, bus routes were performed at peak and non-peak periods, mimicking the routine activity of the population. Mean concentrations of PM_2.5 in the bus and car groups were similar while the fraction of BCe was higher for the bus group. For all routes, mean PM_2.5 concentrations were higher during peak than non-peak hours, with an average of 43.5 ± 33.1 μg m⁻³ and 14.3 ± 10.2 μg m⁻³, respectively. The trace elements S, K and Na originated mainly from vehicle emissions; Na was associated with the presence of biofuel in diesel. Toxic elements (Pb, Cr, Cu, Ni, Zn, Mn) were found at low levels as evident by the total hazard index that ranged from 2.15 × 10⁻⁰³ to 1.38 for volunteers. For all routes, the hazard index ranged from 2.25 × 10⁻⁰³ to 5.03. Average PM_2.5 respiratory deposition dose was estimated to be 0.60 μg/kg-hour for peak hours. Potential health damages to people during their movements and at workplaces close to the traffic were identified. Improvements in the design of the building to reduce the entrance of air pollutants as well as the use of filters in the buses could help to limit population exposure.     

Correlation between automotive CO, HC, NO, and PM emission factors from on-road remote sensing: implications for inspection and maintenance programs

Carbon monoxide (CO), hydrocarbon (HC), and nitrogen oxide (NO) emission factors (EFs) are measured with a commercial vehicle emissions remote sensing system (VERSS) during a large-scale vehicle exhaust emissions study in Las Vegas. Particulate matter (PM) EFs are simultaneously measured for individual vehicles with a newly developed PM-VERSS based on ultraviolet backscatter light detection and ranging (Lidar). The effectiveness of CO and HC EFs as proxy for NO and PM EFs for spark-ignition vehicles is evaluated. Poor correlations were found between EFs for pollutants on an individual vehicle basis indicating that high EFs for one or more pollutants cannot be used as a predictor of high EFs for other pollutants. Stronger functional relationships became evident after averaging the EF data in bins based on rank-order of a single pollutant EF. Low overlap between the highest 10% emitters for CO, HC, NO, and PM was found. These results imply that for an effective reduction of the four pollutants, inspection and maintenance (I/M) programs, including clean screening, should measure all four pollutants individually. Fleet average CO and HC concentrations determined by gaseous VERSS were compared with fleet average CO and HC concentrations measured at low-idle and at high-idle during local I/M tests for spark-ignition vehicles. The fleet average CO concentrations measured by I/M tests at either idle were about half of those measured by remote sensing. The fleet average high-idle HC concentration measured by I/M tests was about half of that measured by VERSS while low-idle I/M and VERSS HC average concentrations were in better agreement. For a typical vehicle trip, most of the fuel is burned during non-idle conditions. I/M measurements collected during idling conditions may not be a good indicator of a vehicle’s potential to be a high emitter. VERSS measurements, when the vehicle is under a load, should more effectively identify high emitting vehicles that have a large contribution to the mobile emissions inventory.     

Development of an emissions inventory model for mobile sources

Traffic represents one of the largest sources of primary air pollutants in urban areas. As a consequence, numerous abatement strategies are being pursued to decrease the ambient concentrations of a wide range of pollutants. A mutual characteristic of most of these strategies is a requirement for accurate data on both the quantity and spatial distribution of emissions to air in the form of an atmospheric emissions inventory database. In the case of traffic pollution, such an inventory must be compiled using activity statistics and emission factors for a wide range of vehicle types. The majority of inventories are compiled using ‘passive’ data from either surveys or transportation models and by their very nature tend to be out-of-date by the time they are compiled. Current trends are towards integrating urban traffic control systems and assessments of the environmental effects of motor vehicles. In this paper, a methodology for estimating emissions from mobile sources using real-time data is described. This methodology is used to calculate emissions of sulphur dioxide (SO₂), oxides of nitrogen (NO_x), carbon monoxide (CO), volatile organic compounds (VOC), particulate matter less than 10 μm aerodynamic diameter (PM₁₀), 1,3-butadiene (C₄H₆) and benzene (C₆H₆) at a test junction in Dublin. Traffic data, which are required on a street-by-street basis, is obtained from induction loops and closed circuit televisions (CCTV) as well as statistical data. The observed traffic data are compared to simulated data from a travel demand model. As a test case, an emissions inventory is compiled for a heavily trafficked signalized junction in an urban environment using the measured data. In order that the model may be validated, the predicted emissions are employed in a dispersion model along with local meteorological conditions and site geometry. The resultant pollutant concentrations are compared to average ambient kerbside conditions measured simultaneously with on-line air quality monitoring equipment.